What the appropriate CFS value is for fishing on a stream is going to vary by fisherperson. I remember fishing Spring a few years ago and thought conditions were ideal (maybe 110cfs or something like that). Another person commented they preferred 70cfs or below. I was streamer fishing, the other angler preferred to use dries.
Given the thousands of miles of streams in PA, and the much smaller number of gauges, the best you can do is figure out which gauge can be a sort of measuring stick for other streams in an area. For instance, I know that if one gauge is about 300cfs, another stream nearby is going to be perfect (more or less - it depends if the 300cfs is a momentary spike from a thunderstorm, which means a much tighter window on when conditions are ideal). But again, it depends on how you are angling, so the spread on "advisable for angling" could be quite large. Larger streams will lag their tributaries, so six hours before a stream falls to 300cfs might be ideal on a tributary.
Bottom line - make it a habit to check out gauges on streams you fish that have them. File the cfs away and also try to correlate a given cfs (and the conditions that led up to that cfs) to other streams. And then you'll know, better than any website that tells you ideal conditions when to fish..