I agree with Chaz. The PAFBC/PASDA has a list of the streams supporting wild trout, which is insanely extensive. Combine that with the Class A and B listings and the wilderness streams, and you can fish for a long time. Almost all of these streams will have brookies, and if you are catching browns, go upstream and you will start catching brookies most of the time. Get out and fish the streams that feed these, or that lie near by. I've discovered a ton of small streams that I'm sure feed brookies up the in mountains walking miles of wild trout waters. These are not listed, but I have fished some of them and pulled some nice brookies. Many times a stream that looks small where it flows in to the main water will have pools etc holding fish further up. I like to find water that I know holds brookies, or is near known water, and check out the water flow on low and high days, and check the elevation change etc to help me predict which streams to check out. I've found some duds that I thought would be good, but more often than not I find some nice little streams and a healthy population of fish. The best part about finding these small "blue liners" is that few other people fish them, so the fish are likely untouched (and aggressive) and all the more fun to catch as well. Not to mention the populations are likely thriving if there is little pressure.
I checked out the PSU data a few days ago, and I agree, it seems like it's a predictor of stream conditions that support the trout. That doesn't guarantee that there are fish there, but it can't hurt. I don't see the need for it, however, when there are already so many resources for streams if you look for them. Then again, I'm all for additional resources because I get half the fun of fishing from hiking/scouting out new streams. I don't like to hit the same stream too often so I'm always out checking out new stuff.